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English: Carrier thermalization in perovskites. 2D electronic spectroscopy (2DES) kinetic at 655 nm pump and 695 nm probe wavelength, which is on the right side of the 2DES map diagonal and thus between the pump wavelength and the bandgap (excitation density: 2 × 10^18 cm^−3). We observe three different regimes: a coherent regime at negative times during which we observe spectral oscillations, a thermalization regime during which we observe a rise in signal much slower than the temporal width of the instrument response function and delayed relative to the rise of the diagonal, and a carrier cooling regime during which the signal slowly decays.
Date
Source Richter, Johannes M.; Branchi, Federico; Valduga de Almeida Camargo, Franco; Zhao, Baodan; Friend, Richard H.; Cerullo, Giulio; Deschler, Felix (2017-08-29). "Ultrafast carrier thermalization in lead iodide perovskite probed with two-dimensional electronic spectroscopy". Nature Communications. 8 (1): 376. doi:10.1038/s41467-017-00546-z. ISSN 2041-1723. PMC 5575115. PMID 28851862.
Author

Johannes M. Richter, Federico Branchi, Franco Valduga de Almeida Camargo, Baodan Zhao,

Richard H. Friend, Giulio Cerullo & Felix Deschler
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29 August 2017

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Date/TimeThumbnailDimensionsUserComment
current13:06, 9 July 2025Thumbnail for version as of 13:06, 9 July 2025687 × 574 (27 KB)Annika of NineFile:Carrier thermalization in perovskites.webp cropped 51 % horizontally, 57 % vertically, 79 % areawise using CropTool with precise mode.

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