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English: Carrier relaxation probed with 2D electronic spectroscopy. a–c 2DES maps for time delays t 2 of a 0 fs, b 80 fs and c 500 fs for an excitation density of 2 × 1018 cm−3. The diagonal of the 2DES maps is indicated with orange lines. d Schematic illustration of carrier relaxation processes. Initially, a non-thermal carrier energy distribution is excited. After undergoing carrier-carrier scattering, carriers form a thermalized distribution with a temperature higher than the lattice. Through carrier-phonon scattering, the carriers subsequently cool down until they reach an equilibrium with the lattice temperature
Date
Source Richter, J.M., Branchi, F., Valduga de Almeida Camargo, F. et al. Ultrafast carrier thermalization in lead iodide perovskite probed with two-dimensional electronic spectroscopy. Nat Commun 8, 376 (2017). https://doi.org/10.1038/s41467-017-00546-z
Author Johannes M. Richter, Federico Branchi, Franco Valduga de Almeida Camargo, Baodan Zhao, Richard H. Friend, Giulio Cerullo & Felix Deschler
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Carrier relaxation probed with 2D electronic spectroscopy.

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29 August 2017

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current13:11, 8 July 2025Thumbnail for version as of 13:11, 8 July 20251,575 × 1,036 (120 KB)Annika of NineUploaded a work by Johannes M. Richter, Federico Branchi, Franco Valduga de Almeida Camargo, Baodan Zhao, Richard H. Friend, Giulio Cerullo & Felix Deschler from Richter, J.M., Branchi, F., Valduga de Almeida Camargo, F. et al. Ultrafast carrier thermalization in lead iodide perovskite probed with two-dimensional electronic spectroscopy. Nat Commun 8, 376 (2017). https://doi.org/10.1038/s41467-017-00546-z with UploadWizard
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